72-223/2008
Titlu proiect
OBTINEREA
DE MATERIALE CU CARACTERISTICI IMBUNATATITE PENTRU TEHNOLOGII NUCLEARE
Coordonator/director
proiect
CO:
Institutul National pentru Fizica Laserilor, Plasmei si Radiatiei/Director
proiect: Dr. Cristian P. LUNGU
Parteneri în
consorţiu
P1. Regia Autonoma de
Activitati Nucleare –Sucursala Cercetari Nucleare
P2. Universitatea Al.I.Cuza Iasi
P3. Universitatea Bucuresti
P4. Universitatea Tehnica de Constructii Bucuresti
P5. Universitatea Ovidius Constanta
P6. Universitatea POLITEHNICA Bucuresti –
Centrul de Cercetari de Biomateriale (BIOMAT)
P7 Institutul national
pentru Fizica si Inginerie Nucleara (IFIN-HH)
Buget/cofinantare:
2.000.000/56.000 lei
Adresa web
www.CAPACIF.inflpr.ro
Obiectivul/rezultatul final al
proiectului Elementele de noutate ale proiectului Beneficiarii rezultatelor
Stadiul de realizare Participare tineri cercetatori Diseminari
Diseminari Etapa 3 Participare tineri
cercetatori
Obiectivul/rezultatul final al proiectului
Scopul general al proiectului
este imbunatatirea domeniului stiintei materialelor prin dezvoltarea de noi metode de caracterizare
a structurilor la nivel microscopic, obtinerea de acoperiri compozite cu
comportare imbunatatita la coroziune, uzura, tribocoroziune, dezvoltarea de noi tehnologii de
fabricatie, noi modele teoretice referitoare la procese si structuri, noi programe
de calcul pentru evaluarea relatiei intre structura filmelor subtiri,
proprietatile lor mecanice si fizice si parametrii plasmelor in tehnologice.
Rezultat final: Dezvoltarea tehnologiei arcului termoionic in vid pentru realizarea depunerilor combinatoriele
ale materialelor de interes pentru reactoarele de fuziune (W, C, Be) cu grosimi
cuprinse intre 0.1 si 10 mm
Elementele de noutate ale proiectului,
originalitate
Prin prezentul proiect se propune dezvoltarea
unei metode originale de simulare a depunerii combinatoriale a stratelor
subtiri care se formeaza in urma actiunii plasmelor de fuziune asupra
materialelor care acopera peretii interiori ai instalatiei de fuziune ITER. Metoda,
bazata pe experienta acumulata la INFLPR in cadrul proiectelor CERES, CEEX
si FP6-EURATOM, asa cum este
descrisa de exemplu in (C. P. Lungu,
I. Mustata, G. Musa, A. M. Lungu, V. Zaroschi, K. Iwasaki, R. Tanaka, Y.
Matsumura, I. Iwanaga, H. Tanaka, T. Oi, K. Fujita: Formation of
nanostructureed Re-Cr-Ni diffusion barrier coatings on Nb superalloys by TVA
method, Surf and
Coat. Techn, Vol.200, 399-402, 2005) consta din generarea
simultana a unor plasme in vaporii materialelor de interes prin producerea electronilor
prin emisie termica la catozii de wolfram, accelerarea lor puternica catre 2
anozi situati la cativa milimetri de acestia (la cateva mii de volti),
concentratrea lor pe anozi, evaporarea intensa a materialelor anodice (in vid
de ordinul a 10‑6 torr) si formarea unor plasme in atomii
evaporati care se extind in spatiu ajungand la substrat unde se depun cu viteze
de ordinul nanometrilor/sec, in straturi formate din combinatii de materiale
pure (fiind evaporate in vid), compacte (ca rezultat al depunerii atom cu atom
beneficiind si de bombardamentul cu ioni energetici ce vin din plasma), fara
incluziuni gazoase.
Beneficiarii rezultatelor, potentialul de aplicare in economie
Rezultatele
Proiectului (Baza de Cunostinte, obtinere de materiale cu caracteristici
imbunatatite pentru tehnologii nucleare, noi
tehnici de procesare a materialelor) vor fi valorificate prin abordarea unor
proiecte noi in cadrul programelor europene FP7 EURATOM-FUZIUNE, asistenta
tehnica catre Societatea Nationala Nuclearelectrica – Fabrica de
Combustibil Nuclear Mioveni, Pitesti
si prin asistarea mediului de afaceri intern (IMM MEDAPTEH SRL, IMM MGM
STAR SRL, OPTICOAT), cat si European (Heikki Sipila
Oy, Finlanda), in dezvoltarea de aplicatii in domenii nenucleare.
Stadiul de realizare (etape
conform planului de realizare cu mentionarea clara a precursorilor
indicatorilor de rezultat cf. HG475/2007):
o
Etapa 1:
§
Buget de stat: 104716 lei
§
Cofinantare: -
§
Precursori*/rezultate intermediare
7 documentatii efectuate de CO si 6 dintre partenerii din
consortiu privind elaborarea modelului de evaporare cu distributie graduala a
concentratiilor a doua materiale pentru formarea de acoperiri
combinatoriale/identificarea tipurilor de materiale, structuri si procese care
pot fi investigate cu resursele actuale ale consortiului.
§
Achizitii realizate: -
o
Etapa 2:
§
Buget de stat: 64085 lei
§
Cofinantare: 17500
lei
§
Precursori*/rezultate intermediare:
8 documentatii efectuate de CO si 7 dintre partenerii din
consortiu privind “Depuneri
preliminare de filme din C si
W”. Caracterizari preliminare ale plasmei si filmelor de C si W.
§
Achizitii realizate: Componenta sistem electrochimic, 17.500 lei
Participare tineri cercetatori (inclusiv specializari/stagii de
formare/doctorate post-doc pe tematica proiectului).
De la INFLPR: 2 tineri cercetatori/ doctoranzi, unul cu
dubla coordonare (Romania/Germania: Alexandru Anghel), au efectuat stagii de
formare de cate 5 luni in Germania (C. Porosnicu si A. Anghel : caracterizare
structurala si din punct de vedere al retentiei de H si D a filmelor din C, W, Be, depuse prin
metoda TVA.
Diseminari/valorificari: Brevete, articole publicate/acceptate spre
publicare (ISI, reviste), carti publicate/acceptate spre publicare, comunicari
stiintifice:
Brevete
Nr. Crt. |
Titlul |
Autori |
Stadiul
brevetarii |
1 |
Dispozitiv de obtinere a unei densităţi stationare de vapori
din materiale cu punct de topire ridicat, |
Autori: R. Vladoiu, V.
Ciupina Victor, G. Musa, C.P. Lungu, V. Zaroschi |
Cerere inregistrare
brevet: Nr. A 00648/20.08.2009 OSIM |
Cărti
Nr. Crt. |
Titlul contributiei |
Autori |
Titlu volum/Editori |
1 |
Nanostructured film
preparation by thermionic vacuum arc,
pp.67-96. |
C.P.Lungu |
New applications of micro- and
nanotechnologies/ Editors: Maria Zaharescu, Liviu ISBN 978-973-27-1803-2 |
Articole ISI
Nr. Crt. |
Titlul |
Autori |
Revista/Index/Volum |
1 |
Surface morphology
influence on deuterium retention in beryllium films prepared by thermionic
vacuum arc method. Pp. 426-429 |
A. Anghel, C.
Porosnicu, M. Badulescu, I. Mustata, C.P. Lungu, K. Sugiyama, S. Lindig, K.
Krieger, J. Roth, A. Nastuta, G. Rusu, G. Popa, |
Nuclear Instruments and
Methods in Physics Research Section B: Beam Interactions with Materials and
Atoms/ Index SCIE ( Science
Citation Index-Expanded)/ Volume 267, Issue 2, January 2009/Elsevier ISSN 0168-583X ISI impact factor:
0.999 |
2 |
Influence of the bias voltage
on the formation of beryllium films by a thermionic vacuum arc method, Pages 242-245 |
Anghel, I. Mustata, C.
Porosnicu, C. P. Lungu, |
Journal of Nuclear Materials/Index SCIE ( Science Citation Index-Expanded)
/ Volume 385, Issue 2, 31 March 2009/Elsevier ISSN 0022-3115, ISI impact factor: 1.501 |
3 |
Determining the radial distribution of the emission
coefficient from a plasma source |
C. Gavrila, |
Optoelectronics and Advanced Materials- Rapid
Communications/ Index SCIE ( Science Citation Index-Expanded)
Vol. 3, No. 8, August 2009, p. 835 – 838, ISSN 1842-6573 |
4 |
„Surface Energy Evaluation of Unhydrogenated
DLC Thin Film Deposited by Thermionic Vacuum Arc (TVA) Method”, |
R. Vladoiu, V. Dinca, G. Musa |
Eur. Phys. J. D/ Index SCIE ( Science Citation Index-Expanded)/
Vol 54, 433 – 437 (2009) |
5 |
Arc
plasma tailoring for the synthesis of compact Tungsten films, |
M. Badulescu, I. Gruia, C. Surdu-Bob, C.
Iacob |
Optoelectronics and Advanced Materials- Rapid
Communications/ Index SCIE ( Science Citation Index-Expanded)/Vol. 3, No. 11, November 2009, p. 1231 - 1234 |
6 |
Characterization of nano-structured carbon-metal
bilayers deposited by Thermionic Vacuum Arc (TVA) techno-logy, Chem. Listy,
102 s1533-s1535 (2008) |
R. Vladoiu, V.Ciupina, C.P.Lungu, O.I.Pompilian,
P.Chiru, A.M.Lungu, G.Prodan, A.Mandes, G.Musa |
Chem. Listy/ Index BDI/ Vol 102/ Chemicke
listy, ISSN 1213-7103 Factor de impact:
0.593 |
Articole publicate in reviste de
specialitate
Nr. Crt. |
Titlul |
Autori |
Revista/volum |
1 |
Preparation and Characterization of Multifunctional, Nanostructured
Coatings Using Thermionic Vacuum Arc Method, pp.1-6 |
Cristian P. Lungu, |
Frontier of Applied Plasma Technology/ Vol.2 July 2009, pp1-6. (Edited by |
2 |
Thermionic vacuum
arc diagnostic using emissive probe, p.147 – 149 |
Tiron, C.
Aniculaesei, G. Popa |
Journal of
Automation, Mobile Robotics and Intelligent Systems,
Index BAZTECH, Polonia/Vol. 3, No. 4, (2009) Editor: Industrial Research
Institute for Automation and Measurements, |
3 |
Electrical and optical diagnostic of the thermionic vacuum arc, |
C. Aniculaesei, A. V. Nastuta, V. Tiron, G. Popa, |
Revista Ştiinţifică “Vasile Adamachi” 2009
ISSN 1221- 9363 |
4 |
thermionic vacuum
arc – plasma and deposited thin films characterisation |
V. Nastuta, C. Aniculaesei, V. Tiron, G. Popa, |
Revista Ştiinţifică “Vasile Adamachi” 2009
ISSN 1221-9363 |
Conferinte
Nr. Crt. |
Titlul |
Autori |
Conferinta
la care s-a comunicat lucrarea |
1 |
Combinatorial Carbon-Tungsten
Film preparation by thermionic vacuum arc method |
C. P.
Lungu, A. M. Lungu, O. Pompilian, C. Porosnicu, R. Vladoiu, G. Prodan, V.
Ciupina, M. Osiac, M.Ganciu, P. Chapon |
E-MRS
2009 Spring Meeting, June 8-12, 2009, |
2 |
Morphological and Compositional
Study on Be-C/Be-W Composite Films Prepared By Thermoinic Vacuum Arc Method |
C.
Porosnicu, A. Anghel, C. P. Lungu, |
E-MRS
2009 Spring Meeting, June 8-12, 2009, |
3 |
Structure and Tribological
Properties of Carbon Based Nanocomposites Grown by TVA Method, |
R.
Vladoiu, V. Ciupina, M. Contulov, A. Mandes, V. Dinca, G.Prodan, C.P. Lungu |
E-MRS
2009 Spring Meeting, June 8-12, 2009, |
4 |
|
A.
Anghel, C.porosnicu, C.P.Lungu, |
. E-MRS 2009 Spring Meeting, June 8-12,
2009, |
5 |
Thermionic Vacuum Arc Plasma Oscillations
Influences on Carbon Film Deposition |
C. Porosnicu, C.
Ticos, I. Jepu, I. Mustata, C. P. Lungu, C. E. A. Grigorescu, V. Andrei, |
E-MRS 2009 Spring Meeting, June 8-12, 2009, |
6 |
TEM
characterization of carbon-tungsten thin films deposited by Thermionic Vacuum
Arc (TVA) technology |
V. Ciupina,
R. Vladoiu, G. Prodan, A. Mandes,
C. P. Lungu, |
”Nanotech
Insight 2009, |
7 |
Ternary
Be-C-W system formation usin thermionic vacuum arc method |
C. P. Lungu, C.
Porosnicu, A. Anghel, C. Luculescu, I. Mustata, AA. M. Lungu, P. Chiru, V.
Zaroschi, D. Dudu,I. Vata, V. Andrei |
10th
International Balkan Workshop on Applied Physics, July 6-8th, 2009, |
8 |
Carbon based nanostructures: synthesis and characterization |
V. Ciupina, I. Morjan, R. Alexandrescu, F. Dumitrache,
G. Prodan, C.P.Lungu, R.Vladoiu, I. Mustata, V. Zaroschi, J. Sullivan, S.
O’Saied, E. Vasile, I.M. Oancea Stanescu, M. Prodan, D. Manole, A.
Mandes, V. Dinca, M. Contulov |
10th International Balkan Workshop on Applied Physics, July 6-8th, 2009, |
9 |
„Morphological and Structural Characterization of
the C-W Nanocomposites”, |
R. Vladoiu, V.
Ciupina, A. Mandes, M. Contulov, V. Dinca, C. Porsnicu, C. P. Lungu, |
17th Symposium on
Application of Plasma Processes - SAPP, 17 - 22.01.2009, Liptovsky Jan, |
10 |
Beryllium
films coatings for fusion applications |
C. P. Lungu, I. Mustata, V. Zaroschi, A. M.
Lungu, P. Chiru, A. Anghel, C. Porosnicu, I. Jepu, C. Ticos, G. Burcea, V.
Bailescu, G. Dinuta, |
The 15th ICIT Conference with international
participation Progress in cryogenics and isotopes separation, |
11 |
Comparison of the beryllium films prepared
by thermionic vacuum arc and thermal evaporation methods |
C. P. Lungu, I.
Mustata, V. Zaroschi, A.M. Lungu, P. Chiru, A. Anghel, C. Porosnicu, I. Jepu,
V. Bailescu, G. Burcea, G. Dinuta, F. Din, N. Balan, G. Serban |
Proc of. ISPC 19, International
Symposium on Plasma Chemistry, |
Articole publicate in reviste
cotate ISI:
1.C.
Gavrila, V. Petrehus, I.Gruia, Image
reconstruction in optical tomography using Radon transform and it’s
inverse, Proceeding of SPIE, Vol. 7388, 31 Dec. 2009, ISSN: 0277-786X, (ISI).
2.I. M. Oancea-Stanescu, V.
Ciupina, G. Prodan, M.Prodan, A. Caraiane, N. Dulgheru, I. Jepu, C.P.Lungu, Transmission electron microscopy analysis
and electrical measurements of carbon thin films, J.Optoel. and Adv. Materials,
Vol.12 ISS.4- 2010 (April , 2010)p. 824 – 828
3.V. Ciupina, J. Sullivan, S. Saied, R. Vladoiu, G. Prodan, I. M.
Oancea-Stanescu, A. Mandes, M. Contulov, V. Dinca, M. Prodan, and D. Manole, “Synthesis and characterization of
some carbon based nanostructures”, Contrib. Plasma Phys.,
1–8 (2010)/DOI 10.1002 / ctpp. 201010157
4.R. Vladoiu, V. Ciupina, M. Contulov, A. Mandes, V. Dinca, G. Prodan, C.
P. Lungu, “Structure and tribological properties
of carbon based nanocomposites grown by TVA method, J Optoelectron Adv Mater
Vol. 12, No. 3, March 2010, p. 553 – 556
Articole acceptate spre publicare in reviste cotate ISI:
1.
A. Marcu, C. M. Ticos, C.
Grigoriu, I. Jepu, C. Porosnicu, A. M. Lungu, C. P. Lungu, Simultaneous Carbon and Tungsten Thin Film Deposition Using Two
Thermionic Vacuum Arcs, Thin Solid Films, acceptata (2010)
2.
V. Ciupina, R. Vladoiu, C.P.
Lungu, V. Dinca, A. Mandes, M. Contulov, I. M. Oancea-Stranescu, G. Prodan, M.
Prodan, V. Zaroschi, Carbon-tungsten
based nanostructures for fusion systems, Rom. Reports in Phys., acceptata (2010)
3.
V.
Tiron, M. Dobromir, V. Pohoata and G. Popa, Ion energy distribution in thermionic vacuum arc plasma, IEEE Transaction on
Plasma Science, 2010, (acceptata pentru publicare).
4.
V. Tiron,
L. Mihaescu, C. P. Lungu, G. Popa, Strong
double layer structure in thermionic vacuum arc plasma, Romanian
Journal of Physics, 2010, (acceptata pentru publicare).
Reviste internationale necotate ISI:
1.C. Gavrila, V. Petrehus, I.Gruia, Using Radon Transform in Image Reconstruction, Scientific Journal Mathematical Modelling in Civil Engineering, Vol.6, nr.3 sept. 2010, ISSN: 2066-6926 (B+).
2.V. Tiron and G. Popa, “Control of the thermionic vacuum arc plasma”, 24th International Symposium on Discharges and Electrical Insulation in Vacuum, Conference proceedings, Volume II, p. 391- 394, 2010.
Carti:
1.C. P. Lungu, I. Mustaţă, C, C.Porosnicu, I. Jepu, A. Anghel– Caracterizarea filmelor compozite combinatoriale obţinute prin metoda arcului termoionic în vid, Bucureşti, Editura Academiei Oamenilor de Ştiinţă din România, 2010, ISBN 978-606-92500-1-3
Reviste din Romania:
1. R. Vladoiu, V. Ciupina, A. Mandes,
M.Contulov, V.Dinca, C.P.Lungu, Tribological
properties of carbon-tungsten nanocomposites synthetized by thermionic vacuum
arc (TVA) method, Revista AOSR, acceptata (2010)
Conferinte internationale:
12. R. Vladoiu, V. Ciupina, A. Mandes, V. Dinca, M. Contulov, G. Musa, „Structural and morphological properties of
the carbon based nanostructures deposited by Gaseous Thermoionic Vacuum Arc (GTVA)
method”, International Conference E-MRS 2010, June
7-11 (2010) Strasbourg, France
13. R.
Vladoiu, M. Contulov, V. Ciupina, M. Prodan and G. Musa, “Deposition
of Nanostructures Hydrogenated Carbon Thin
Films by Decomposition of Methane using G-TVA Method”, 15th Conference on Plasma Physics and
Applications (CPPA2010), July 1-4
(2010)
14. R.
Vladoiu, V. Ciupina, C. P. Lungu, V. Dinca, A. Mandes, “Growth and characterization of the C-Si nanocomposites using
thermionic vacuum arc (TVA) method”, IBWAP 2010, July 7-9 (2010) Constanta, Romania
15. A. Chirila, R. Vladoiu,
V. Ciupina, Influence of the Substrate on the
Mechanical Properties in the Carbon Thin Films Deposited by Thermionic Vacuum
Arc (TVA) Technology, ISCBPU-8, September 3 - 5
(2010) Constanta, Romania
Conferinte nationale:
2. V. Ciupina,
R. Vladoiu, A. Mandes, M. Contulov, M. Prodan, V. Zaroschi, C. P. Lungu, Nanostructured C-Me thin films grown by
Thermionic Vacuum Arc (TVA) method for high adhesion coatings”, Conferinţa Naţională de
Fizică (CNF) 2010, September 23-25 2010, Iaşi, Romania
3. V. Ciupina, I. Morjan, R. Alexandrescu, R.
Vladoiu, I.M. Oancea-Stanescu, V. Dinca, G. Prodan, Carbon based nanostructures with industrial applications - Conferinţa Naţională de
Fizică (CNF) 2010, September 23-25 2010, Iaşi, Romania
Lucrari invitate:
2. R. Vladoiu, V. Ciupina, C. P. Lungu, Characterization of carbon-tungsten nanocomposites synthetized by
Thermionic Vacuum Arc (TVA) method, International
conference (E-MRS 2010), Strasbourg,
France, June 7-11, (2010)
3. R. Vladoiu, V. Ciupina, M. Contulov, A. Mandes, V. Dinca, M. Prodan, Properties of the nanostructured carbon thin films deposited by G-TVA method in methane plasma”, IBWAP 2010, Constanta, Romania, July 7-9, (2010)
4. R.
Vladoiu, Nanostructures Based on
Carbon Obtained by Different Configurations of the Thermionic Vacuum Arc (TVA)
Method”, ISCBPU-8, September 3 - 5
Participare la
expozitii, targuri
1. Expoziţia realizărilor
cercetării româneşti SALONUL CERCETĂRII – 2010, Complexul
Expoziţional ROMEXPO, 6 – 9 octombrie 2010, Pavilionul 13, DOMENII: 2.X Nanomateriale, Nanotehnologii; (Filme nanostructurate multifunctionale: filme magnetorezistive, filme cu
coeficient de frecare redusa, filme pentru celule solare, filme carbonice,
filme pentru aplicatii in fuziune)
2. Târgul Industrial Internaţional HANNOVER MESSE, Tehnologie TVA pentru depuneri filme carbonice cu legaturi tip diamant, 16-20 aprilie 2010.
Brevet:
1. Metoda pentru producerea filmelor compozite din carbon-wolfram cu arc termoionic in vid, autori C. P. Lungu, C. Porosnicu, I. Jepu, C. Ticos, A. Marcu, I. Mustata, V. Zaroschi, V. Tiron, G. Popa, R. Vladoiu, V.Ciupina, Inregistrare OSIM: A/00912 din 28.09.2010
1.
Corneliu Porosnicu: Stagiu de cercetare stiintifica la Institutu
de de Fizica Plasmei (IPP-Garching), Garching, Germania, in perioada 1.03 - 31.05.
2010 (INFLPR)
2.
Alexandru Anghel: Stagiu de cercetare stiintifica (4 luni) la Institutul
de de Fizica Plasmei (IPP-Garching), Garching, Germania, in perioadele 1.02-
30.04. 2010, 15.08 – 15.09.2010 (INFLPR)
3.
Mandes Aurelia: Stagiu de cercetare stiintifica la Universitatea
leopold-Franzens, Innsbruck, Austria in perioada 15.04.2010 -15.05.2010 (P5
Univ Ovidius)
4.
Contulov Mirela: Stagiu de cercetare stiintifica la Universitatea
leopold-Franzens, Innsbruck, Austria in perioada 15.04.2010 -15.05.2010 (P5
Univ Ovidius)
5.
Dinca Virginia: Stagiu de cercetare stiintifica la Universitatea
Charles, Praga, Rep. Ceha, in perioada 1.11.2009 -31.01.2010 ( P5 Univ Ovidius)
6.
Pompilian Oana: Stagiu de doctorat la Universitatea Lile, Franta
(15 sept 2009 – 15 sept 2011)